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Jeong Haeyun,Ki Hosung,Kim Jong Goo,Kim Jungmin,Lee Yunbeom,Ihee Hyotcherl 대한화학회 2022 Bulletin of the Korean Chemical Society Vol.43 No.3
Time-resolved x-ray liquidography (TRXL) is a powerful technique to study molecular structural dynamics in the solution phase. Typically, a TRXL experiment is conducted during limited beamtime at a beamline of a synchrotron or an x-ray free-electron laser, demanding a proper design and careful planning. In this regard, the optimal q range needs to be determined to find the optimal x-ray energy and sample-to-detector distance. For such purpose, here, we present effective ways to quantify the sensitivity of the TRXL data as a function of q to various factors such as the atomic positions, internuclear distances, solvent cage, and bulk solvent. The developed approaches are also applicable to other types of time-resolved diffraction, such as ultrafast electron diffraction.
Ichiyanagi, K.,Sato, T.,Nozawa, S.,Kim, K. H.,Lee, J. H.,Choi, J.,Tomita, A.,Ichikawa, H.,Adachi, S.,Ihee, H.,Koshihara, S. International Union of Crystallography 2009 Journal of synchrotron radiation Vol.16 No.3
<▼1><P>A new method of time-resolved solution scattering utilizing X-ray multilayer optics is presented.</P></▼1><▼2><P>100 ps time-resolved X-ray solution-scattering capabilities have been developed using multilayer optics at the beamline NW14A, Photon Factory Advanced Ring, KEK. X-ray pulses with an energy bandwidth of Δ<I>E</I>/<I>E</I> = 1–5% are generated by reflecting X-ray pulses (Δ<I>E</I>/<I>E</I> = 15%) through multilayer optics, made of W/B<SUB>4</SUB>C or depth-graded Ru/C on silicon substrate. This tailor-made wide-bandwidth X-ray pulse provides high-quality solution-scattering data for obtaining photo-induced molecular reaction dynamics. The time-resolved solution scattering of CH<SUB>2</SUB>I<SUB>2</SUB> in methanol is demonstrated as a typical example.</P></▼2>