Graphene oxide composite hydrogels for wearable devices

다국어 초록 (Multilingual Abstract)

For graphene oxide (GO) composite hydrogels, a two-dimensional GO material is introduced into them, whose special structure is used to improve their properties. GO contains abundant oxygen-containing functional groups, which can improve the mechanical properties of hydrogels and support the application needs. Especially, the unique-conjugated structure of GO can endow or enhance the stimulation response of hydrogels. Therefore, GO composite hydrogels have a great potential in the field of wearable devices. We referred to the works published in recent years, and reviewed from these aspects: (a) structure of GO; (b) factors affecting the mechanical properties of the composite hydrogel, including hydrogen bond, ionic bond, coordination bond and physical crosslinking; (c) stimuli and signals; (d) challenges. Finally, we summarized the research progress of GO composite hydrogels in the field of wearable devices, and put forward some prospects.

참고문헌 (Reference)

1 Ma D, "Wearable, antifreezing, and healable epidermal sensor assembled from longlasting moist conductive nanocomposite organohydrogel" 11 (11): 41701-41709, 2019

2 Hong S, "Wearable thermoelectrics for personalized thermoregulation" 5 (5): 11-, 2019

3 Ates HC, "Wearable devices for the detection of COVID-19" 4 (4): 13-14, 2021

4 Xie Z, "Ultrastretchable, self-healable and adhesive composite organohydrogels with a fast response for human-machine interface applications" 10 (10): 8266-8277, 2022

5 Jin X, "Ultrastretchable, self-adhesive, strain-sensitive and self-healing GO@DA/Alginate/P(AAc-co-AAm)multifunctional hydrogels via musselinspired chemistry" 254 : 117316-, 2021

6 Dai X, "Ultraantifreeze, ultra-stretchable, transparent, and conductive hydrogel for multi-functional flexible electronics as strain sensor and triboelectric nanogenerator" 15 (15): 5461-5468, 2022

7 Li G, "Ultra-stretchable and healable hydrogel-based triboelectric nanogenerators for energy harvesting and self-powered sensing" 11 (11): 17437-17444, 2021

8 Feng S, "Tunable dual temperature-pressure sensing and parameter self-separating based on ionic hydrogel via multisynergistic network design" 11 (11): 21049-21057, 2019

9 Jiang YW, "Topological supramolecular network enabled high-conductivity, stretchable organic bioelectronics" 375 (375): 1411-1417, 2022

10 Yang T, "Thermo-responsive shape memory sensors based on tough, remolding and anti-freezing hydrogels" 8 (8): 2326-2335, 2020

11 Xia S, "The role of reduced graphene oxide as a “2D flexible crosslinking point”in composite hydrogels" 62 (62): 416-425, 2021

12 Kadumudi FB, "The manufacture of unbreakable bionics via multifunctional and self-healing silk-graphene hydrogels" 33 (33): e2100047-, 2021

13 Xiang X, "The composite hydrogel with"2D flexible crosslinking point"of reduced graphene oxide for strain sensor" 2021

14 Dreyer DR, "The chemistry of graphene oxide" 39 (39): 228-240, 2010

15 Xiang Xu ; Zhu Ying ; Gao Changqin ; Du Han ; Guo Chunwen, "Study on the structure of reduced graphene oxide prepared by different reduction methods" 한국탄소학회 32 (32): 557-566, 2022

16 Xiang X, "Study of microwave reduction of graphene oxide suspension : structure and functional groups" 57 (57): 3280-3294, 2022

17 Xiang X, "Study of capacitance type flexible electronic devices based on polyacrylamide and reduced graphene oxide composite hydrogel" 2022

18 Zhang L, "Strong and tough PAm/SA hydrogel with highly strain sensitivity" 10 : 415-, 2022

19 Deng Z, "Stretchable, rapid self-healing guar gum-poly(acrylic acid)hydrogels as wearable strain sensors for human motion detection based on Janus graphene oxide" 191 : 627-636, 2021

20 He F, "Stretchable, biocompatible, and multifunctional silk fibroin-based hydrogels toward wearable strain/pressure sensors and triboelectric nanogenerators" 12 (12): 6442-6450, 2020

21 Zhang H, "Stretchable and conductive composite structural color hydrogel films as bionic electronic skins" 8 (8): e2102156-, 2021

22 Deng Z, "Stimuli-responsive conductive nanocomposite hydrogels with high stretchability, self-healing, adhesiveness, and 3D printability for human motion sensing" 11 (11): 6796-6808, 2019

23 Yang Man ; Chen Yiyang ; Wang Haitao ; Zou Yilun ; Wu Pingxiu ; Zou Jing ; Jiang Jizhou, "Solvothermal preparation of CeO2 nanoparticles–graphene nanocomposites as an electrochemical sensor for sensitive detecting pentachlorophenol" 한국탄소학회 32 (32): 1277-1285, 2022

24 Wang T, "Smart composite hydrogels with pH-responsiveness and electrical conductivity for flexible sensors and logic gates" 2019

25 Ying B, "Skin-like hydrogel devices for wearable sensing" 24 (24): 103174-, 2021

26 Xia M, "Self-powered multifunction ionic skins based on gradient polyelectrolyte hydrogels" 16 (16): 4714-4725, 2022

27 Hsu HH, "Self-powered and plant-wearable hydrogel as LED power supply and sensor for promoting and monitoring plant growth in smart farming" 2021

28 Li W, "Self-powered and high sensitivity ionic skins by using versatile organogel" 2022

29 Taylor DL, "Self-healing hydrogels" 28 (28): 9060-9093, 2016

30 Yang X, "Sandwich-like polypyrrole/reduced graphene oxide nanosheets integrated gelatin hydrogel as mechanically and thermally sensitive skinlike bioelectronics" 2020

31 Liu Guijing ; Shi Yanying ; Wang Lei ; Song Yadong ; Gao Shanmin ; Liu Dong ; Fan Leqing, "Reduced graphene oxide/polypyrrole composite: an advanced electrode for high-performance symmetric/asymmetric supercapacitor" 한국탄소학회 30 (30): 389-397, 2020

32 Sun J, "Recent progress in the tailored growth of two-dimensional hexagonal boron nitride via chemical vapour deposition" 47 (47): 4242-4257, 2018

33 Qin T, "Recent progress in conductive self-healing hydrogels for flexible sensors" 2022

34 Yu W, "Progress in the functional modification of graphene/graphene oxide : a review" 10 (10): 15328-15345, 2020

35 Wei J, "Polyvinyl alcohol/graphene oxide conductive hydrogels via the synergy of freezing and salting out for strain sensors" 2022

36 Zheng X, "Polysaccharide-tackified composite hydrogel for skin-attached sensors" 9 (9): 3343-3351, 2021

37 Gao W, "New insights into the structure and reduction of graphite oxide" 1 (1): 403-408, 2009

38 Chen Z, "Multifunctional conductive hydrogels and their applications as smart wearable devices" 9 (9): 2561-2583, 2021

39 Chen J, "Multifunctional conductive hydrogel/thermochromic elastomer hybrid fibers with a core-shell segmental configuration for wearable strain and temperature sensors" 12 (12): 7565-7574, 2020

40 Li N, "MXenes : An emerging platform for wearable electronics and looking beyond" 4 (4): 377-407, 2021

41 Niu S, "Lowtemperature wearable strain sensor based on a silver nanowires/graphene composite with a near-zero temperature coefficient of resistance" 13 (13): 55307-55318, 2021

42 Zhang Z, "Liquid metal-created macroporous composite hydrogels with self-healing ability and multiple sensations as artificial flexible sensors" 9 (9): 875-883, 2021

43 Sun JY, "Ionic skin" 26 (26): 7608-7614, 2014

44 Jiang J, "Improving stability of MXenes" 15 (15): 6551-6567, 2022

45 Zhang Y, "Highstrength and highly electrically conductive hydrogels for wearable strain sensor" 2021

46 Zhao R, "Highly strong, stretchable, and conductive reduced graphene oxide composite hydrogel-based sensors for motoring strain and pressure" 3 (3): 5155-5161, 2021

47 Chen K, "Highly stretchable, sensitive, and durable Ag/tannic acid@graphene oxide-composite hydrogel for wearable strain sensors" 4 (4): 2036-2046, 2022

48 Mao J, "Highly stretchable, self-healing, and strain-sensitive based on doublecrosslinked nanocomposite hydrogel" 17 : 22-27, 2020

49 Zhang Z, "Highly stretchable porous composite hydrogels with stable conductivity for strain sensing" 2021

50 Li Y, "Highly sensitive and wearable self-powered sensors based on a stretchable hydrogel comprising dynamic hydrogen bond and dual coordination bonds" 2021

51 Xia S, "Highly sensitive and wearable gel-based sensors with a dynamic physically cross-linked structure for strain-stimulus detection over a wide temperature range" 7 (7): 11303-11314, 2019

52 Wang Q, "Highly dispersed graphene network achieved by using a nanoparticle-crosslinked polymer to create a sensitive conductive sensor" 6 (6): 5006-5013, 2019

53 Chen H, "High toughness multifunctional organic hydrogels for flexible strain and temperature sensor" 9 (9): 23243-23255, 2021

54 Wu L, "High stretchable, pH-sensitive and self-adhesive rGO/CMCNa/PAA composite conductive hydrogel with good strain-sensing performance" 2021

55 Hou W, "High performance dual strain-temperature sensor based on alginate nanofibril/graphene oxide/polyacrylamide nanocomposite hydrogel" 2021

56 Zhao R, "Graphene oxide-based composite organohydrogels with high strength and low temperature resistance for strain sensors" 18 (18): 1201-1208, 2022

57 Compton OC, "Graphene oxide, highly reduced graphene oxide, and graphene : versatile building blocks for carbon-based materials" 6 (6): 711-723, 2010

58 Wang Y, "Graphene assisted ion-conductive hydrogel with super sensitivity for strain sensor" 2021

59 Lee SH, "Fully portable continuous real-time auscultation with a soft wearable stethoscope designed for automated disease diagnosis" 8 (8): 12-, 2022

60 Xie Z, "Freezingtolerant, widely detectable and ultra-sensitive composite organohydrogel for multiple sensing applications" 9 (9): 10127-10137, 2021

61 Wu G, "Fabrication of capacitive pressure sensor with extraordinary sensitivity and wide sensing range using PAM/BIS/GO nanocomposite hydrogel and conductive fabric" 2021

62 Kumar M. Infant Shyam ; Kirupavathy S. Shahil ; Shalini S., "Exploration on reduced graphene oxide/strontium pyro niobate electrode material for electrochemical energy storage applications" 한국탄소학회 31 (31): 619-633, 2021

63 Bu Y, "Evolution of layer distance and structural arrangement of graphene oxide with various oxygen content and functional types in low temperature : a ReaxFF molecular dynamics simulation" 2022

64 윤조희 ; 박홍준 ; 박승화 ; 이경균 ; 최봉길, "Electrochemical characterization of reduced graphene oxide as an ion-to-electron transducer and application of screen-printed all-solid-state potassium ion sensors" 한국탄소학회 30 (30): 73-80, 2020

65 Konios D, "Dispersion behaviour of graphene oxide and reduced graphene oxide" 430 : 108-112, 2014

66 Lin R, "Digitally-embroidered liquid metal electronic textiles for wearable wireless systems" 13 (13): 2190-, 2022

67 Mathew Elma Elizaba ; Balachandran Manoj, "Crumpled and porous graphene for supercapacitor applications: a short review" 한국탄소학회 31 (31): 537-555, 2021

68 Amin I, "Covalent polymer functionalization of graphene/graphene oxide and its application as anticorrosion materials" 9 : 032002-, 2022

69 Yin H, "Construction of polydopamine reduced graphene oxide/sodium carboxymethyl cellulose/polyacrylamide double network conductive hydrogel with high stretchable, pH-sensitive and strain-sensing properties" 2022

70 Zhang H, "Conductive hydrogel-based flexible strain sensors with superior chemical stability and stretchability for mechanical sensing in corrosive solvents" 45 (45): 4647-4657, 2021

71 Cho B, "Chemical sensing of 2D graphene/MoS2 heterostructure device" 7 (7): 16775-16780, 2015

72 Liu X, "Cellulose nanocrystal reinforced conductive nanocomposite hydrogel with fast selfhealing and self-adhesive properties for human motion sensing" 2021

73 Gao Q, "Bioinspired stimuli-responsive hydrogel with reversible switching and fluorescence behavior served as light-controlled soft actuators" 2021

74 Jing X, "Biocompatible, self-healing, highly stretchable polyacrylic acid/reduced graphene oxide nanocomposite hydrogel sensors via musselinspired chemistry" 136 : 63-72, 2018

75 Zhang J, "Antibacterial, antifreezing, stretchable, and self-Healing organohydrogel electrode based triboelectric nanogenerator for self-powered biomechanical sensing" 2022

76 Hu K, "A tough organohydrogel-based multiresponsive sensor for a triboelectric nanogenerator and supercapacitor toward wearable intelligent devices" 10 (10): 12092-12103, 2022

77 Novoselov KS, "A roadmap for graphene" 490 (490): 192-200, 2012

78 Rahmani P, "A review on the features, performance and potential applications of hydrogel-based wearable strain/pressure sensors" 298 : 102553-, 2021

79 Su Y, "A multifunctional hydrogel fabricated via ultra-fast polymerization by graphene oxide-adsorbed liquid metal nanodroplets" 2022

80 Wang M, "A fast self-healing and conductive nanocomposite hydrogel as soft strain sensor" 567 : 139-149, 2019

81 Pan X, "A bionic tactile plastic hydrogel-based electronic skin constructed by a nerve-like nanonetwork combining stretchable, compliant, and self-healing properties" 2020