다중이용시설 내 PM2.5 중 PAHs 농도분포 특성 = Characteristics of Polycyclic Aromatic Hydrocarbons from PM2.5 in the Public Facilities

다국어 초록 (Multilingual Abstract)

This study was performed in the 48 selected public facilities in three metropolitan cities (Seoul, Daejeon, and Kwangjoo) and three general cities (Suncheon, Gwangyang, and Yeosu) to measure of the characteristics from May to October 2011. Air samples (PM2.5) were collected at the indoor and outdoor places for 24-hrs using the mini volume air sampler and analyzed 24 gaseous and particulate polycyclic aromatic hydrocarbons (PAHs) through the GC/MS. The recoveries of gaseous and particulate PAHs ranged between 60.7% to 127.2% and 57.7% to 132.5% respectively and its relative standard deviation (RSD) was 11.1%. This QA/QC results about the were adequate for the Korean national standards. The concentration levels of the PAHs in present study were acenaphthene > dibenz(a,h)anthracene > benzo(g,h,i)perylene > 3-methylcholanthrene > indeno[1,2,3-cd]pyrene for the particulate PAHs in the 48 selected public facilities. In the case of acenaphthene, the mean concentration showed the highest levels of 22.42 ng/㎥ and 34.57 ng/㎥ in the level of gaseous and particulate phase, respectively. The total PAHs concentration for the PC room is the highest in surveyed public facilities of this study and the smoking/non smoking ratio in the PC room was 3.45. This results indicated that smoking in the PC room is seemed to play a major source and the effective risk management strategies were needed to minimize or eliminate the public health effect for customers in the PC room.

목차 (Table of Contents)

• Abstract
• 1. 서 론
• 2. 연구내용 및 방법
• 3. 결과 및 고찰
• 4. 결 론
• Acknowledgments
• References

참고문헌 (Reference)

1 손부순, "일부 주부의 실내공기 중 PAHs 노출에 관한 연구" 한국환경과학회 16 (16): 323-331, 2007

2 홍상범, "수도권 지역 PM10의 PAHs 농도 특성" 한국대기환경학회 25 (25): 347-359, 2009

3 WHO, "WHO guidelines for indoor air quality : selected pollutants"

4 Dubowsky, S.D., "The contribution of traffic to indoor concentrations of PAHs, Expos" 9 : 312-321, 1999

5 Rogge, W.F., "Source of organic aerosols. 8. Boilers burning no. 2 distillate fuel oil" 31 : 2731-2737, 1997

6 Harrison, R.M., "Source apportionment of atmospheric PAHs collected from an urban location in Birmigham, UK" 30 : 825-832, 1996

7 Simcik, M.F., "Source apportionment and source/sink relationship of PAHs in the coastal environment of Chicago and Lake Michigan" 33 : 5071-5079, 1999

8 Zhou, J., "Size distribution of PAHs in urban and suburban sites of Beijing, China" 61 : 792-799, 2005

9 Ohura, T., "Simultaneous liquid chromatographic determination of 39 polycyclic aromatic hydrocarbons in indoor and outdoor air and application to a survey on indoor air pollution in Fuji, Japan" 85 (85): 188-202, 2002

10 US EPA, "Provisional Guidance for Quantitative Risk Assessment of Polycyclic Aromatic Hydrocarbons"

11 Ohura, T., "Prediction of personal exposure to PM2.5 and carcinogenic polycyclic aromatic hydrocarbons by their concentrations in residential microenvironments" 39 (39): 5592-5599, 2005

12 US EPA, "Polynuclear Aromatic Hydrocarbons"

13 Stumpe-Vısna, I., "Polycyclic aromatic hydrocarbons in meat smoked with different types of wood" 110 : 794-797, 2008

14 Ohura, T., "Polycyclic aromatic hydrocarbons in indoor and outdoor environments and factors affecting their concentrations" 38 : 77-83, 2004

15 Orecchio, S., "Polycyclic aromatic hydrocarbons (PAHs) in indoor emission from decorative candles" 45 : 1888-1895, 2011

16 Lu, H., "Pollution patterns of polycyclic aromatic hydrocarbons in tobacco smoke" 139 : 193-198, 2007

17 Zhu, L., "Pollution level, phase distribution and source analysis of polycyclic aromatic hydrocarbons in residential air in Hangzhou, China" 162 (162): 1165-1170, 2009

18 Titcombe, M.E., "Personal and indoor exposure to PM2.5 and polycyclic aromatic hydrocarbons in the southern highlands of Tanzania: a pilot-scale study" 2010

19 Lau, C., "Levels of selected organic compounds in materials for candle productions and humans exposures to candle emissions" 34 : 1623-1630, 1997

20 US EPA, "Integrated Risk Information System, Washington DC, last revised March"

21 International Agency for Research on Cancer(IARC), "IARC Monographs on the Evaluation of the Carcinogenic Risks to Humans, 32" 33-451, 1983

22 MOE, "Establishment of the policy infrastructure for integrated risk management of environmental media" 2009

23 National Institute of Environmental Research, "Environmental standard method for air quality(ES 01552.1), PAHs-GC/MC"

24 Oanh, N.T.K., "Emission of PAHs and particulate matter from domestic combustion of selected fuels" 33 : 2703-2709, 1999

25 Back, S,O., "Effect of Ambient Temperature on the Distribution of Atmospheric Concentrations of Polycyclic Aromatic Hydrocarbons in the Vapor and Particulate Phases" 14 (14): 117-131, 1998

26 Whitehead, T., "Determinants of polycyclic aromatic hydrocarbon levels in house dust" 21 (21): 123-132, 2011

27 Lung, S.C., "Customers' exposure to PM2.5 and polycyclic aromatic hydrocarbons in smoking/nonsmoking sections of 24-h coffee shops in Taiwan" 14 (14): 529-535, 2004

28 US EPA, "Compendium of methods TO-15. Determination of volatile organic compounds (VOCs) in air collected in specially-prepared canisters and analyzed by gas chromatography/ mass spectrometry (GC/MS) 2nd Ed"

29 US EPA, "Compendium of methods TO-13A. Determination of polycyclic aromatic hydrocarbons (PAHs) in ambient air using gas chromatography/ mass spectrometry (GC/MS),2ndEd"

30 Masih, J., "Characterristics of polycyclic aromatic hydrocarbons in indoor and outdoor atmospheric in the North central part of India" 177 (177): 190-198, 2010

31 Durlak, S.K., "Characterization of PAHs particulate and gaseous emissions from polystyrene combustion" 32 : 2301-2307, 1998

32 Marr, L.C.W., "Characterization of PAHs in motor vehicle fuels and exhaust emission" 33 : 3091-3099, 1999

33 Park, S.S., "Atmospheric PAHs in Seoul, Korea" 36 : 2917-2924, 2002

34 Miller, R.M., "Assessment of benzo( a)pyrene-equivalent carcinogenicity and mutagenicity of residential indoor versus outdoor polycyclic aromatic hydrocarbons exposing young children in New York City" 7 (7): 1889-1900, 2010

35 WHO, "Air Auality Guidelines Global Update"

36 National Institute of Environmental Research, "A study on management of non-regulated indoor air pollutant in Korea (Ⅲ)" 2011

37 National Institute of Environmental Research, "A study on Research of Hazardous Air Pollutants(HAPs) in Yeosu and Gwangyang Area" 2009

38 National Institute of Environmental Research, "A study on Research of Hazardous Air Pollutants(HAPs) in Ulsan Area" 2010

39 National Institute of Environmental Research, "A study on Research of Hazardous Air Pollutants(HAPs) in Daesan" 2012