<P><B>Abstract</B></P> <P>With emerging stability issues in fuel cell technology, a non-conventional catalyst not supported on carbon materials has been highlighted because it can avoid negative influences of carbon supp...
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https://www.riss.kr/link?id=A107435702
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2017
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SCI,SCIE,SCOPUS
학술저널
16-22(7쪽)
0
상세조회0
다운로드다국어 초록 (Multilingual Abstract)
<P><B>Abstract</B></P> <P>With emerging stability issues in fuel cell technology, a non-conventional catalyst not supported on carbon materials has been highlighted because it can avoid negative influences of carbon supp...
<P><B>Abstract</B></P> <P>With emerging stability issues in fuel cell technology, a non-conventional catalyst not supported on carbon materials has been highlighted because it can avoid negative influences of carbon support materials on the stability, such as carbon corrosion. The nanostructured thin film catalyst is representative of non-conventional catalysts, which shows improved stability, enhanced mass specific activity, and fast mass transfer at high current densities. However, the nanostructured thin film catalyst usually requires multi-step processes for fabrication, making its mass production complex and irreproducible. We introduce a Pt-Cu alloy nanostructured thin film catalyst, which can be simply prepared by electrodeposition. By using hydrogen bubbles as a template, a three-dimensional free-standing foam of Cu was electrodeposited directly on the micro-porous layer/carbon paper and it was then displaced with Pt by simple immersion. The structure characterization revealed that a porous thin Pt-Cu alloy catalyst layer was successfully formed on the micro-porous layer/carbon paper. The synthesized Pt-Cu alloy catalyst exhibited superior durability compared to a conventional Pt/C in single cell test.</P> <P><B>Highlights</B></P> <P> <UL> <LI> A Pt-Cu alloy foam catalyst was synthesized directly on micro porous layer (MPL). </LI> <LI> A foam structure was prepared on MPL by Cu electrodeposition using bubble template. </LI> <LI> The Pt-Cu alloy was formed by Pt displacement following the electrodeposition. </LI> <LI> The Pt-C alloy/MPL catalyst showed superior durability to Pt/C in single cell test. </LI> </UL> </P>