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An All-Solid-State Li-Ion Battery with a Pre-Lithiated Si-Ti-Ni Alloy Anode
Yersak, Thomas A.,Son, Seoung-Bum,Cho, Jong Soo,Suh, Soon-Sung,Kim, Young-Ugk,Moon, Jeong-Tak,Oh, Kyu Hwan,Lee, Se-Hee The Electrochemical Society 2013 Journal of the Electrochemical Society Vol.160 No.9
<P>In this paper we demonstrate an all-solid-state Li-ion battery with a specific energy of 225 mWh g<SUP>−1</SUP> based upon the combined mass of both the composite anode and cathode. To realize this full cell, we pair an iron sulfide and sulfur composite cathode with a Si-based anode. The anode active material is a Si-Ti-Ni alloy with good ionic and electronic conductivity that attains a stable specific capacity of 400 mAh g<SUP>−1</SUP> based upon the total mass of the composite anode. To our knowledge, this is the highest stable Si-based all-solid-state anode specific capacity reported to date. To utilize both a lithium free anode and cathode, we adopt a pre-lithiation technique involving stabilized lithium metal powder. This is the first time that this technique has been demonstrated in an all-solid-state battery.</P>
Conformal Coatings of Cyclized-PAN for Mechanically Resilient Si nano-Composite Anodes
Piper, Daniela Molina,Yersak, Thomas A.,Son, Seoung-Bum,Kim, Seul Cham,Kang, Chan Soon,Oh, Kyu Hwan,Ban, Chunmei,Dillon, Anne C.,Lee, Se-Hee Wiley Blackwell (John Wiley Sons) 2013 ADVANCED ENERGY MATERIALS Vol.3 No.6