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Yongkui Yang,Yifeng Ling,Longfei Wang,Peizhe Sun,Lin Zhao,Hongyang Wang 한국화학공학회 2023 Korean Journal of Chemical Engineering Vol.40 No.5
With rapid industrialization and population growth, sewage sludge generation has increased worldwide, and it needs to be treated properly. The pyrolysis of sewage sludge into biochar provides sustainable benefits for concomitant pollutant adsorption and waste treatment. Sulfamethoxazole (SMX) antibiotics are highly prevalent in waste-water owing to their widespread utilization and low metabolic rate and removal efficiency during conventional waste-water treatment. Biochar is known to effectively remove pollutants from wastewater. However, the adsorption capacity and mechanism of SMX adsorption onto sludge-based biochar are currently unclear. Therefore, the adsorption behavior of SMX on sludge-based biochar from three sources (raw sludge, compost sludge, and digested sludge) and ZnCl2-modified biochar was investigated. Among the unmodified biochars, raw sludge-based biochar exhibited the highest adsorption capacity, followed by compost sludge-based and digested sludge-based biochar. The pore-forming effect of ZnCl2 application significantly increased the biochar specific surface area, which increased the equilibrium adsorption of SMX from 6.1 mg/g to 49.3 mg/g. The adsorption mechanisms involved electrostatic interactions, pore filling, hydrophobic interactions, hydrogen bonding, and π-π interactions. The findings of this study demonstrate the development of sewage sludge biochar and its effectiveness for the treatment of antibiotics containing wastewater.
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Wang Yongkui,Huang Xiaochen,Zhou Jiafeng,Fang Jun,Gao Yan,Ge Jinlong,Miao Shu,Xie Zhuoming 한국원자력학회 2023 Nuclear Engineering and Technology Vol.55 No.2
In this work, pure W and W-0.5wt%HfC alloy (WHC05) were fabricated by sintering and hot-rolling following the same processing route. After exposing to a high flux deuterium plasma irradiation with the Dþ flux to three fluences of 6.00 1024, 2.70 1025 and 7.02 1025 D/m2, the evolution of surface morphology, deuterium retention and hardening behaviors in pureWand WHC05 has been studied. The SEM results show the formation of D blisters on the irradiated area, and with the increase of D implantation, the size of these blisters increases from 200 ~ 500 nm (2.70 1025 D/m2) to 1 ~ 2 mm (7.02 1025 D/m2) in WHC05 and from 1 ~ 2 mm (2.70 1025 D/m2) to > 3 mm (7.02 1025 D/m2) in pure W, respectively. A higher D retention and obvious hardening are observed in pure W than that of the WHC05 alloy, indicating an improve radiation resistance in WHC05 compared to pure W.
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