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- 검색키워드
- 저자 : Tran Dang Thanh (검색결과 93 건)
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Tran Dang Thanh,Phan, T. L.,Nguyen Van Chien,Do Hung Manh,Yu, S. C. IEEE 2014 IEEE transactions on magnetics Vol.50 No.4
<P>In this paper, we present a detailed study of the magnetocaloric effect and critical properties around the ferromagnetic-paramagnetic (FM-PM) phase transition of La<SUB>0.7</SUB>Ca<SUB>0.3-x</SUB>Sr<SUB>x</SUB>MnO<SUB>3</SUB> nanoparticles with x = 0.10, 0.11, and 0.12. The samples were synthesized by a combination of reactive milling and thermal processing. The average crystallite size of nanoparticles estimated from the linewidth of X-ray diffraction peaks by using the Williamson-Hall method is about 50 nm. Under a magnetic field change of 10 kOe, the maximum magnetic entropy change (|ΔS<SUB>max</SUB>|) reaches values of 1.47, 1.42, and 1.38 J·kg<SUP>-1</SUP>·K<SUP>-1</SUP> for x = 0.10, 0.11, and 0.12, respectively, at around 300 K. The refrigerant capacity is thus in between 44 and 54 J·kg<SUP>-1</SUP>. Particularly, the M<SUP>2</SUP> versus H/M curves prove that all the samples exhibit a second-order magnetic phase transition. Based on Landau's phase-transition theory and careful analyses of the magnetic data around the FM-PM transition region, we have determined the critical exponents β, y, δ, and T<SUB>C</SUB>. Here, the β values obtained are 0.397, 0.453, and 0.456 for x = 0.10, 0.11, and 0.12, respectively, which are in between those expected on the basis of the mean-field theory (β = 0.5) and value of the 3-D Heisenberg model (β = 0.365). The result proves the coexistence of shortand long-range FM interactions in La<SUB>0.7</SUB>Ca<SUB>0.3-x</SUB>Sr<SUB>x</SUB>MnO<SUB>3</SUB> nanoparticles. The nature of this phenomenon is discussed thoroughly.</P>
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Thanh, Tran Dang,Linh, Dinh Chi,Yen, Pham Duc Huyen,Bau, Le Viet,Ky, Vu Hong,Wang, Zhihao,Piao, Hong-Guang,An, Nguyen Manh,Yu, Seong-Cho Elsevier 2018 PHYSICA B-CONDENSED MATTER - Vol.532 No.-
<P><B>Abstract</B></P> <P>In this work, we present a detailed study on the magnetic properties and the magnetocaloric effect (MCE) of La<SUB>1−x</SUB>K<SUB>x</SUB>MnO<SUB>3</SUB> compounds with <I>x</I>=0.05–0.2. Our results pointed out that the Curie temperature (<I>T</I> <SUB>C</SUB>) could be controlled easily from 213 to 306K by increasing K-doping concentration (<I>x</I>) from 0.05 to 0.2. In the paramagnetic region, the inverse of the susceptibility can be analyzed by using the Curie-Weiss law, <I>χ</I>(<I>T</I>)=<I>C</I>/(<I>T</I>−<I>θ</I>). The results have proved an existence of ferromagnetic clusters at temperatures above <I>T</I> <SUB>C</SUB>. Based on Banerjee's criteria, we also pointed out that the samples are the second-order phase transition materials. Their magnetic entropy change was calculated by using the Maxwell relation and a phenomenological model. Interestingly, the samples with <I>x</I>=0.1–0.2 exhibit a large MCE in a range of 282–306K, which are suitable for room-temperature magnetic refrigeration applications. The composites obtained from single phase samples (<I>x</I>=0.1–0.2) exhibit the high relative cooling power values in a wide temperature range. From the viewpoint of the refrigerant capacity, the composites formed out of La<SUB>1−x</SUB>K<SUB>x</SUB>MnO<SUB>3</SUB> will become more useful for magnetic refrigeration applications around room-temperature.</P>
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Magnetic Properties and Magnetocaloric Effect at Room Temperature of Ni50−xAgxMn37Sn13 Alloys
Tran Dang Thanh,Nguyen Thi Mai,Nguyen Huy Dan,The-Long Phan,유성초 한국물리학회 2014 THE JOURNAL OF THE KOREAN PHYSICAL SOCIETY Vol.65 No.10
In this work, we present a detailed study of the magnetic properties and the magnetocaloric effectat room temperature of Ni50−xAgxMn37Sn13 alloys with x = 1, 2, and 4, which were prepared byusing an arc-melting method. Experimental results reveal that a partial replacement of Ag for Nileads to a decrease in the anti-FM phase in the alloys. In addition, the martensitic-austenitic phasetransition shifts towards lower temperature and is broaded. The Curie temperature (TAC ) for theaustenitic phase also shifts toward to lower temperature, but not by much. The Curie temperaturewas found to be 308, 305, and 298 K for x = 1, 2, and 4, respectively. The magnetic entropychange (Sm) of the samples was calculated by using isothermal magnetization data. Under anapplied magnetic field change of 10 kOe, the maximum value of Sm (|Smax|) was achieved ataround room temperature and did not change much (0.8 J·kg−1·K−1) with increasing Ag-dopingconcentration. Particularly, the M2 vs. H/M curves prove that all the samples exhibited a secondordermagnetic phase transition. Based on Landau’s phase-transition theory and careful analyses ofthe magnetic data around the TAC , we have determined the critical parameters ,, , and TC. Theresults show that the values are located between those expected for the 3D-Heisenberg model (= 0.365) and mean-field theory ( = 0.5). Such a result proves the coexistence of short-range andlong-range ferromagnetic interactions in Ni50−xAgxMn37Sn13 alloys. The nature of the changes inthe critical parameters and the |Smax| is thoroughly discussed by means of structural analyses.
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Thanh, Tran Dang,Xuan Hau, Kieu,Huyen Yen, Pham Duc,Manh, T. V.,Yu, S. C.,Phan, T. L.,Telegin, A.,Telegin, S.,Naumov, S. IEEE 2018 IEEE transactions on magnetics Vol.54 No.11
<P>In this paper, we present a detailed analysis on the critical behavior of La<SUB>1.2</SUB>Sr<SUB>1.8</SUB>Mn<SUB>2</SUB>O<SUB>7</SUB> single crystal via isothermal magnetization measured at different temperatures around the paramagnetic–ferromagnetic phase transition at <TEX>$T_{C} = 85$</TEX> K. Using the Landau–Lifshitz coefficients, the Arrott plots ( <TEX>$H/M = a(T) + b(T)M^{2}$</TEX>) of sample have been analyzed. It showed that a(T) changed from positive to negative values at different temperatures in the field ranges of <TEX>$H = 0$</TEX>–10, 10–30, and 30–50 kOe, indicating that the critical behavior could not be described with a single model under different applied fields. Through the modified Arrott plots method, the Kouvel–Fisher method, and the critical isotherm analysis, we determined the values of the critical exponents for La<SUB>1.2</SUB>Sr<SUB>1.8</SUB>Mn<SUB>2</SUB>O<SUB>7</SUB> around its magnetic phase transition over different magnetic field ranges. The critical exponent <TEX>$\beta $</TEX> value is found to be 0.501, 0.417, and 0.371 under field ranges of <TEX>$H = 0$</TEX>–10, 10–30, and 30–50 kOe, respectively. This means that the <TEX>$\beta $</TEX> value depends strongly on the strength of the applied field, shifting from the value approaching that of the mean field model ( <TEX>$\beta = 0.5$</TEX>) to the 3-D-Heisenbeg model ( <TEX>$\beta = 0.365$</TEX>). Meanwhile, its <TEX>$\gamma $</TEX> value is quite stable ( <TEX>$\gamma =0.973$</TEX>–1.074), almost independent on the choice of field fitting range. In addition, using the reduced temperature <TEX>$\varepsilon = (T-T_{C}$</TEX>)/ <TEX>$T_{C}$</TEX> and the obtained critical exponents, almost <TEX>$M(H, T$</TEX>) data measured near <TEX>$T_{C}$</TEX> obey the scaling equation <TEX>$M(H, \varepsilon) = \varepsilon ^{\boldsymbol {\beta }}f_{\pm }(H/\varepsilon ^{\boldsymbol {\beta +\gamma }}$</TEX>), where <TEX>$f_{+}$</TEX> and <TEX>$f_{-}$</TEX> are regular analytic functions corresponding to data at <TEX>$T > T_{C}$</TEX> and <TEX>$T < T_{C}$</TEX>, respectively.</P>
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Thanh, Tran Dang,Huyen Yen, Pham Duc,Hau, Kieu Xuan,Bau, Le Viet,Yu, S. C. IEEE 2018 IEEE transactions on magnetics Vol.54 No.11
<P>In this paper, we have investigated the critical properties in the vicinity of the ferromagnetic (FM)–paramagnetic (PM) phase transition in a polycrystalline sample of La<SUB>0.75</SUB>Ca<SUB>0.2</SUB>Ag<SUB>0.05</SUB>MnO<SUB>3</SUB>, which was prepared by a solid-state reaction method. Temperature dependence of the inverse of the susceptibility <TEX>$\chi ^{-1}$</TEX> ( <TEX>$T$</TEX>) proves an existence of the Griffiths phase well above Curie temperature ( <TEX>$T_{C} = 230$</TEX> K). Detailed analyses of the isothermal magnetization <TEX>$M$</TEX>( <TEX>$H$</TEX>, <TEX>$T$</TEX>) data reveal the sample exhibiting a second-order magnetic phase transition, and its temperature dependences of the saturation magnetization and the initial susceptibility obey the asymptotic relations. Using the modified Arrott plots method, the Kouvel–Fisher method, and the critical isotherm analysis, the critical parameters ( <TEX>$\beta$</TEX>, <TEX>$\gamma$</TEX>, <TEX>$\delta$</TEX>, and <TEX>$T_{C}$</TEX>) of La<SUB>0.75</SUB>Ca<SUB>0.2</SUB>Ag<SUB>0.05</SUB>MnO<SUB>3</SUB> compound have been estimated. Using these critical exponent values, almost <TEX>$M$</TEX>( <TEX>$H$</TEX>, <TEX>$T$</TEX>) data measured at different temperatures around FM–PM phase transition are collapsed onto two universal curves of <TEX>$M/\vert \varepsilon \vert ^{\boldsymbol {\beta }}$</TEX> versus <TEX>$H/\vert \varepsilon \vert ^{\boldsymbol {\beta }+\boldsymbol {\gamma }}$</TEX> corresponding to the regular functions for <TEX>$T > T_{C}$</TEX> and <TEX>$T < T_{C}$</TEX>, respectively.</P>
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Tran Dang Thanh,Phan, T. L.,Le Mai Oanh,Nguyen Van Minh,Jong Suk Lee,Yu, S. C. IEEE 2014 IEEE transactions on magnetics Vol.50 No.6
<P>This paper presents the influence of Mn doping on the structural characterization, and optical and magnetic properties of SrTi<SUB>1-x</SUB>Mn<SUB>x</SUB>O<SUB>3</SUB>(x = 0.0-0.1) materials prepared by a solid-state reaction method. The detailed analyses of X-ray diffraction patterns indicate an incorporation of Mn dopants into Ti sites of the SrTiO<SUB>3</SUB> host lattice. There is a cubic to tetragonal transformation, which takes place at a threshold concentration x ≈ 0.04. The optical absorption spectra show a rapid increase in the absorption coefficient. The bandgap energy (Eg) related to the direct electron transition decreases with increasing Mn concentration: Eg decreases from 3.15 eV for x = 0 to 1.28 eV for x = 0.10. From this point of view, the SrTi<SUB>1-x</SUB>Mn<SUB>x</SUB>O<SUB>3</SUB> materials are considered as promising materials for photocatalytic applications. Interestingly, while the samples with x = 0.0-0.02 are diamagnetic, the others with x = 0.04-0.10 exhibit weak ferromagnetism. The ferromagnetic order increases with increasing Mn concentration. Based on the results of structural and optical analyses, the nature of magnetism in the samples is explained thoroughly.</P>
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Tran Dang Thanh,Phan, T. L.,Phung Quoc Thanh,Hoang Nam Nhat,Duong Anh Tuan,Yu, S. C. IEEE 2014 IEEE transactions on magnetics Vol.50 No.6
<P>This paper presents a detailed study on the Co-doping influence on the electrical and magnetotransport properties of La0.7Ca0.3Mn1-xCoxO3(x = 0.09-0.17) prepared by solid-state reaction. Magnetic measurements versus temperature revealed a gradual decrease of the magnetization (M) and Curie temperature (T-C) with increasing Co concentration (x). The T-C values vary from 194 to 159 K as changing x from 0.09 to 0.17, respectively. H/M versus M-2 performances around T-C prove the x = 0.09 sample undergoing a first-order magnetic phase transition (FOMT) while the samples with x >= 0.11 undergo a second-order magnetic phase transition (SOMT). The other with x = 0.10 is considered as a threshold concentration of the FOMT-SOMT transformation. Considering temperature dependences of resistivity, rho(T), in the presence and absence of the magnetic field, the samples (excepting for x = 0.17) exhibit a metal-insulator transition at T (P) = 60-160 K, which shifts toward lower temperatures with increasing x. In the metallic-ferromagnetic region, the rho(T) data are well fitted to a power function rho(T) = rho(0) + rho(2) T-2 + rho(4.5) T-4.5. This indicates electron-electron and electron-magnon scattering processes are dominant at temperatures T < T (P). In addition, the conduction data at temperatures T > theta(D)/2 (theta(D) is the Debye temperature) and T (P) < T < theta(D)/2 obey the small-polaron and variable-range hopping models, respectively. The values of activation energy E-p, and density of states at the Fermi level N(E-F) were accordingly determined. Here, N(E-F) increases while E-p decreases when an external magnetic field is applied. We also have found that N(E-F) increases when materials transfer from the FOMT to the SOMT, and N(E-F) value becomes smallest for the sample having the coexistence of the FOMT and SOMT (i.e., x = 0.10).</P>
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Tran Dang Thanh,Phan, T. L.,Pham Thi Thanh,Nguyen Hai Yen,Nguyen Huy Dan,Yu, S. C. IEEE 2014 IEEE transactions on magnetics Vol.50 No.4
<P>This paper presents the magnetocaloric effect and critical behavior of alloy ingot and ribbon samples of Ni<SUB>50</SUB>Mn<SUB>37</SUB>Sn<SUB>13</SUB> doped with 8% Ag, which were prepared by an arc-melting and rapidly quenched melt-spinning methods, respectively. Experimental results reveal that a partial replacement of Ag for Ni leads to stamping out the antiferromagnetic martensitic phase. This means that there is only the austenitic phase with a ferromagnetic-paramagnetic (FM-PM) phase-transition temperature of T<SUB>C</SUB> ≈ 295 K. Detailed studies and analyses around the phase transition region prove both samples undergoing a second-order magnetic phase transition. Basing on magnetic field dependences of magnetization, we have determined the magnetic-entropy change (ΔS<SUB>m</SUB>) of the samples. Under a field change of 10 kOe, the maximum magnetic-entropy change (|ΔS<SUB>max</SUB>|) reaches values 0.54 and 0.69 J · kg<SUP>-1</SUP> · K<SUP>-1</SUP> for the alloy ingot and ribbon, respectively. Using Landau's phase-transition theory, and careful analyses of the magnetic data around the FM-PM transition region, we have determined the critical parameters (T<SUB>C</SUB>, β, γ, and δ) in the low field range (below 10 kOe) with T<SUB>C</SUB> = 294.8 K, β = 0.469 ± 0.011, γ = 1.149 ± 0.060, and δ = 3.4 ± 0.1 for the alloy ingot, and with T<SUB>C</SUB> = 294.4 K, β = 0.449 ± 0.005, γ = 1.319 ± 0.040, and δ = 3.9 ± 0.1 for the alloy ribbon. One can see that β values fall in between those expected for the 3-D Heisenberg model (β = 0.365) and mean-field theory (β = 0.5). This indicates a coexistence of short-range and long-range FM interactions in both the samples. The nature of changes in value related to the critical parameters and maximum ΔS<SUB>m</SUB> is thoroughly discussed by means of structural analyses.</P>
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