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RISS 인기검색어
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- 저자 : Jianguo Tang (검색결과 5 건)
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Yanxia Xu,Bo Tang,Xingfu Song,Ze Sun,Jianguo Yu 한국화학공학회 2018 Korean Journal of Chemical Engineering Vol.35 No.12
We evaluated the effect of particle size and associated dynamics on a hydrocyclone separation process in order to understand the movement of the particle trajectories inside the hydrocyclone via numerical analysis, with particles of acid hydrolysis residues discharged in TiO2 production via the sulfate method as a case study. The values obtained from the numerical simulation were successfully compared with those from experimental tests in the literature, allowing a description of the dynamics of the particles, their acting forces, and their relevant properties together with separation efficiency. The results showed that particle motion is jointly controlled by the drag force, the pressure gradient force and the centrifugal force. With increasing particle size, the influence of the drag force is weakened, whereas that of the centrifugal force and pressure gradient is strengthened. Factors including particle density, slurry viscosity, and inlet slurry flow rate also contribute to a clear and useful understanding of particle motion behavior in the hydrocyclone as a method for improving the separation efficiency.
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Mechanisms of dry flue-gas desulfurization using natural manganese oxide ores
Yongxiang Chen,Yunjiao LI,Xinlong Cao,Jianguo Li,Sanchuan Tang,Wanqi Ye,Xianzhen Zhang 한국화학공학회 2019 Korean Journal of Chemical Engineering Vol.36 No.7
The mechanisms of flue-gas desulfurization using high and low-grade natural manganese oxide ores were comparatively studied. Both manganese oxide ores exhibit good desulfurization capabilities with SO2 content in the effluents less than 30 ppm, but the low-grade ores show the much better desulfurization capability. XRD and SEM/EDS results reveal that the MnO2 absorbs the SO2 to convert to MnSO4. The SO2 give prior to react with the surface MnO2 and the produced MnSO2 enriched on the surface leads to the gradually decrease of the SO2 removal rate during desulfurization process. The better desulfurization capability of the low-grade ores is ascribed to the more dispersive MnO2 due to the poriferous/lax internal tunnel structure, and the embedded inert SiO2 shows better support effects to avoid pore structure blocking, which is favorable for enhancing the diffusion of the SO2 and desulfurization reaction process. This study is of significance in the comprehensive utilization of the low-grade natural manganese oxide ores, environmental protection and even the preparation of the desulfurization catalyst with MnO2.
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Zhao, Guoqing,Shen, Wenfei,Jeong, Eunwook,Lee, Sang-Geul,Yu, Seung Min,Bae, Tae-Sung,Lee, Gun-Hwan,Han, Seung Zeon,Tang, Jianguo,Choi, Eun-Ae,Yun, Jungheum American Chemical Society 2018 ACS APPLIED MATERIALS & INTERFACES Vol.10 No.32
<P>Improving the wetting ability of Ag on chemically heterogeneous oxides is technically important to fabricate ultrathin, continuous films that would facilitate the minimization of optical and electrical losses to develop qualified transparent Ag film electrodes in the state-of-the-art optoelectronic devices. This goal has yet to be attained, however, because conventional techniques to improve wetting of Ag based on heterogeneous metallic wetting layers are restricted by serious optical losses from wetting layers. Herein, we report on a simple and effective technique based on the partial oxidation of Ag nanoclusters in the early stages of Ag growth. This promotes the rapid evolution of the subsequently deposited pure Ag into a completely continuous layer on the ZnO substrate, as verified by experimental and numerical evidence. The improvement in the Ag wetting ability allows the development of a highly transparent, ultrathin (6 nm) Ag continuous film, exhibiting an average optical transmittance of 94% in the spectral range 400-800 nm and a sheet resistance of 12.5 Ω sq<SUP>-1</SUP>, which would be well-suited for application to an efficient front window electrode for flexible solar cell devices fabricated on polymer substrates.</P> [FIG OMISSION]</BR>
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Shasha Gai,Jiqing Jiao,Wei Wei,Yao Li,Lihua Liu,Yi Liu,Baize Lv,Yao Wang,Laurence A. Bel¯ore,Jianguo Tang 성균관대학교(자연과학캠퍼스) 성균나노과학기술원 2018 NANO Vol.13 No.08
The well-defined NaGdF4:Yb,Er nanorods (NRs) with various aspect ratios were synthesized using a facile hydrothermal method. The morphology and crystal phase of NRs could be controlled by reaction conditions. NaGdF4:Yb,Er NRs with various aspect ratios could be synthesized and their upconversion (UC) luminescence was tuned. It is displayed that the NRs with aspect ratios about 5 exhibited the strongest UC luminescence among samples. The growth mechanism and morphology transition of NRs had been deduced by schematic diagram. And UC mechanism had been determined by energy level diagrams. Compared with previous reports, the work provided a facial method for UCNRs with various aspect ratios at lower temperature.
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Zhao, Guoqing,Shen, Wenfei,Jeong, Eunwook,Lee, Sang-Geul,Chung, Hee-Suk,Bae, Tae-Sung,Bae, Jong-Seong,Lee, Gun-Hwan,Tang, Jianguo,Yun, Jungheum American Chemical Society 2018 ACS APPLIED MATERIALS & INTERFACES Vol.10 No.47
<P>Controlling the shape and crystallography of nanocrystals during the early growth stages of a noble metal layer is important because of its correlation with the final layer morphology and optoelectrical features, but this task is unattainable in vapor deposition processes dominated by artificially uncontrollable thermodynamic free energies. We report on experimental evidence for the controllable evolution of Ag nanocrystals as induced by the addition of nitrogen, presumed to be nonresidual in the Ag lattice given its strong float-out behavior. This atypical formation of energetically stable Ag nanocrystals with significantly improved wetting abilities on a chemically heterogeneous substrate promotes the development of an atomically flat, ultrathin, high-purity Ag layer with a thickness of only 5 nm. This facilitates the fabrication of Ag thin-film electrodes exhibiting highly enhanced optical transparency over a broad spectral range in the visible and near-infrared spectral range. An Ag thin-film electrode with a ZnO/Ag/ZnO configuration exhibits an average transmittance of about 95% in the spectral range of 400-800 nm with a maximum transmittance of over 98% at 580 nm, which is comparable with the best transparency values so far reported for transparent electrodes. This degree of optical transparency provides an excellent chance to improve the photon absorption of photovoltaic devices employing an Ag thin film as their window electrode. This is clearly confirmed by the superior performance of a flexible organic solar cell with a power conversion efficiency of 8.0%, which is far superior to that of the same solar cell using a conventional amorphous indium tin oxide electrode (6.4%).</P> [FIG OMISSION]</BR>
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