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Orientation dependence of the fracture behavior of graphene
Jhon, Y.I.,Jhon, Y.M.,Yeom, G.Y.,Jhon, M.S. Pergamon Press ; Elsevier Science Ltd 2014 Carbon Vol.66 No.-
Graphene has unique mechanical properties in that it is simultaneously very strong and stretchy, which severely hampers the prediction of its orientation-dependent fracture behavior based on conventional theories used for common brittle or ductile materials. For the first time, by exploring the entire range of available tensile orientations, this study reveals the unique anisotropic fracture response of graphene using molecular dynamics simulations. We found that, as the uniaxial tensile direction rotates from armchair (0<SUP>o</SUP>) to zigzag orientation (30<SUP>o</SUP>), both the tensile strength and strain remain almost constant up to an orientation angle of ~12<SUP>o</SUP>, then they rapidly increase (exponential growth), resulting in a remarkable degradation of the tensile strength compared to brittle fracture counterpart (inverse-sinusoidal growth). This typical fracture pattern holds for 100-700K. We propose a model that can explain its physical origin in good agreement with the simulation results. We also found that the elastic behavior of graphene is quasi-isotropic for all tensile orientations, in contrast to its anisotropic fracture behavior. Using indentation simulations of graphene, we showed that the anisotropic/isotropic features of fracture/elasticity are also well-preserved in the two-dimensional tensile systems but its fracture anisotropicity is greatly attenuated due to the inherent sixfold symmetry of graphene.
The mechanical responses of tilted and non-tilted grain boundaries in graphene
Jhon, Y.I.,Zhu, S.E.,Ahn, J.H.,Jhon, M.S. Pergamon Press ; Elsevier Science Ltd 2012 Carbon Vol.50 No.10
Various mechanical characteristics of tilted and non-tilted grain boundaries in graphene were investigated under tension and compression in directions perpendicular and parallel to the grain boundaries using molecular dynamics simulation. In contrast to the non-tilted grain boundary and the pristine graphene, the mechanical response of tilted grain boundary was observed to be quite unique under perpendicular tension, exhibiting distinct crack propagation prior to tensile failure and the subsequent pattern of incomplete fracture. These features are manifested as a remarkable decrease in the slope and a rugged pattern in the stress-strain curves. The characteristic of incomplete fracture was striking especially for large misorientation angles with formation of long monoatomic carbon chains, suggesting a methodology for feasible production of the monoatomic carbon chains that have been difficult to synthesize and extract. Under perpendicular compression, the folding of the sheet occurred consistently along grain boundaries during the entire process, indicating a tunable folding, while the folding line wandered extensively for pristine graphene. Under parallel compression, we found that folding along grain boundaries disturbed the bending of the graphene substantially for intrinsic reinforcement.
Highly Selective and Low Damage Etching of GaAs/AlGaAs Heterostructure using Cl2/O2 Neutral Beam
Park, B. J.,Yeon, J. K.,Lim, W. S.,Kang, S. K.,Bae, J. W.,Yeom, G. Y.,Jhon, M. S.,Shin, S. H.,Chang, K. S.,Song, J. I.,Lee, Y. T.,Jang, J. H. Springer-Verlag 2010 Plasma chemistry and plasma processing Vol.30 No.5