http://chineseinput.net/에서 pinyin(병음)방식으로 중국어를 변환할 수 있습니다.
변환된 중국어를 복사하여 사용하시면 됩니다.
Why hybrid porous solids capture greenhouse gases?
Fé,rey, Gé,rard,Serre, Christian,Devic, Thomas,Maurin, Guillaume,Jobic, Hervé,Llewellyn, Philip L.,De Weireld, Guy,Vimont, Alexandre,Daturi, Marco,Chang, Jong-San Royal Society of Chemistry 2011 Chemical Society reviews Vol.40 No.2
<P>Hybrid porous solids, with their tunable structures, their multifunctional properties and their numerous applications, are currently topical, particularly in the domain of adsorption and storage of greenhouse gases. Most of the data reported so far concern the performances of these solids in this domain, particularly in terms of adsorbed amounts of gas but do not explain at the atomic level why and how adsorption and storage occur. From a combination of structural, spectroscopic, thermodynamic experiments and of molecular simulations, this <I>tutorial review</I> proposes answers to these open questions with a special emphasis on CO<SUB>2</SUB> and CH<SUB>4</SUB> storage by some rigid and flexible hybrid porous materials.</P> <P>Graphic Abstract</P><P>Why and how hybrid porous solids capture gases: exploration combining appropriate <I>in situ</I> measurements and molecular simulations. <IMG SRC='http://pubs.rsc.org/services/images/RSCpubs.ePlatform.Service.FreeContent.ImageService.svc/ImageService/image/GA?id=c0cs00040j'> </P>
Permyakova, Anastasia,Skrylnyk, Oleksandr,Courbon, Emilie,Affram, Maame,Wang, Sujing,Lee, U-Hwang,Valekar, Anil H.,Nouar, Farid,Mouchaham, Georges,Devic, Thomas,De Weireld, Guy,Chang, Jong-San,Steunou WILEY-VCH 2017 CHEM SUS CHEM Vol.10 No.7
<P>The energy-storage capacities of a series of water-stable porous metal-organic frameworks, based on high-valence metal cations (Al3+, Fe3+, Cr3+, Ti4+, Zr4+) and polycarboxylate linkers, were evaluated under the typical conditions of seasonal energy-storage devices. The results showed that the microporous hydrophilic Al-dicarboxylate MIL-160(Al) exhibited one of the best performances. To assess the properties of this material for space-heating applications on a laboratory pilot scale with an open reactor, a new synthetic route involving safer, greener conditions was developed. This led to the production of MIL-160(Al) on a 400g scale, before the material was shaped into pellets through a wet-granulation method. The material exhibited a very high energy-storage capacity for a physical-sorption material (343Whkg(-1)), which is in full agreement with the predicted value.</P>