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- 저자 : ( Dongkyu Lee ) (검색결과 405 건)
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Exciton dynamics in cation-exchanged CdSe/PbSe nanorods: The role of defects
Lee, Sooho,Wang, Yimeng,Liu, Yawei,Lee, Dongkyu,Lee, Kangha,Lee, Doh C.,Lian, Tianquan Elsevier 2017 Chemical physics letters Vol.683 No.-
<P>Cation exchange occurs via defect initiated solid-state diffusion, a process that can lead to defect formations. The effect of such inherent defect formation on carrier dynamics of cation-exchanged heterostructures remains poorly understood. Herein, we report exciton dynamics in type II CdSe/PbSe heterostructure nanorods formed via cation exchange. The majority of electrons in CdSe domains decays in 5 ps due to ultrafast carrier trapping. The defect generated by cation exchange can be healed by annealing the as-synthesized CdSe/PbSe heterostructure nanorods. This study suggests a strategy for improving properties of heteronanostructures prepared by cation exchange for applications in photovoltaics and photocatalysis. (C) 2017 Elsevier B.V. All rights reserved.</P>
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Direct Cd-to-Pb Exchange of CdSe Nanorods into PbSe/CdSe Axial Heterojunction Nanorods
Lee, Dongkyu,Kim, Whi Dong,Lee, Seokwon,Bae, Wan Ki,Lee, Sangheon,Lee, Doh C. American Chemical Society 2015 Chemistry of materials Vol.27 No.15
<P>We report synthesis of PbSe nanorods (NRs) and PbSe/CdSe axial heterojunction NRs via direct Cd-to-Pb cation exchange in CdSe NRs. Use of suited ligand–cation combinations enables the cation exchange while keeping the nanomaterial morphology intact. For example, solvation of Cd<SUP>2+</SUP> using oleylamine (OLA) allows for the cation exchange process, which would not be possible by using oleic acid instead of OLA. A mild cation exchange process, such as mixing Pb-oleate and OLA with CdSe NRs at 130 or 150 °C, results in anisotropic replacement of CdSe into PbSe along the ⟨0001⟩ direction of wurtzite CdSe, and a partial conversion leads to the formation of heterostructure NRs containing axial CdSe/PbSe heterojunctions. While the cation exchange proceeds at both tips of CdSe NRs, exchange appears to be faster on (0001̅) planes. Binding energy calculation based on density functional theory reveals that OLA binds strongly to the (0001̅) facet of CdSe NRs, leading to asymmetric cation exchange. This protocol to convert CdSe nanocrystals directly into PbSe broadens the design range of CdSe/PbSe heterojunction nanomaterials potentially with various morphologies because template CdSe nanocrystals can be prepared in different shapes via colloidal synthesis.</P><P><B>Graphic Abstract</B> <IMG SRC='http://pubs.acs.org/appl/literatum/publisher/achs/journals/content/cmatex/2015/cmatex.2015.27.issue-15/acs.chemmater.5b01548/production/images/medium/cm-2015-01548m_0006.gif'></P><P><A href='http://pubs.acs.org/doi/suppl/10.1021/cm5b01548'>ACS Electronic Supporting Info</A></P>
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Jeong, Hyun Woo,Lee, Joo-Won,Kim, Woo Sik,Choe, Sung Sik,Kim, Kyung-Hee,Park, Ho Seon,Shin, Hyun Jung,Lee, Gha Young,Shin, Dongkyu,Lee, Hanjae,Lee, Jun Hee,Choi, Eun Bok,Lee, Hyeon Kyu,Chung, Heekyoun American Diabetes Association 2011 Diabetes Vol.60 No.2
<P><B>OBJECTIVE</B></P><P>Peroxisome proliferator–activated receptor (PPAR)-α/γ dual agonists have been developed to alleviate metabolic disorders. However, several PPARα/γ dual agonists are accompanied with unwanted side effects, including body weight gain, edema, and tissue failure. This study investigated the effects of a novel PPARα/γ dual agonist, CG301269, on metabolic disorders both in vitro and in vivo.</P><P><B>RESEARCH DESIGN AND METHODS</B></P><P>Function of CG301269 as a PPARα/γ dual agonist was assessed in vitro by luciferase reporter assay, mammalian one-hybrid assay, and analyses of PPAR target genes. In vitro profiles on fatty acid oxidation and inflammatory responses were acquired by fatty acid oxidation assay and quantitative (q)RT-PCR of proinflammatory genes. In vivo effect of CG301269 was examined in <I>db/db</I> mice. Total body weight and various tissue weights were measured, and hepatic lipid profiles were analyzed. Systemic glucose and insulin tolerance were measured, and the in vivo effect of CG301269 on metabolic genes and proinflammatory genes was examined by qRT-PCR.</P><P><B>RESULTS</B></P><P>CG301269 selectively stimulated the transcriptional activities of PPARα and PPARγ. CG301269 enhanced fatty acid oxidation in vitro and ameliorated insulin resistance and hyperlipidemia in vivo. In <I>db/db</I> mice, CG301269 reduced inflammatory responses and fatty liver, without body weight gain.</P><P><B>CONCLUSIONS</B></P><P>We demonstrate that CG301269 exhibits beneficial effects on glucose and lipid metabolism by simultaneous activation of both PPARα and PPARγ. Our data suggest that CG301269 would be a potential lead compound against obesity and related metabolic disorders.</P>
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Wang, Nianfang,Koh, Sungjun,Jeong, Byeong Guk,Lee, Dongkyu,Kim, Whi Dong,Park, Kyoungwon,Nam, Min Ki,Lee, Kangha,Kim, Yewon,Lee, Baek-Hee,Lee, Kangtaek,Bae, Wan Ki,Lee, Doh C IOP 2017 Nanotechnology Vol.28 No.18
<P>We present facile synthesis of bright CdS/CdSe/CdS@SiO<SUB>2</SUB> nanoparticles with 72% of quantum yields (QYs) retaining ca 80% of the original QYs. The main innovative point is the utilization of the highly luminescent CdS/CdSe/CdS seed/spherical quantum well/shell (SQW) as silica coating seeds. The significance of inorganic semiconductor shell passivation and structure design of quantum dots (QDs) for obtaining bright QD@SiO<SUB>2</SUB> is demonstrated by applying silica encapsulation via reverse microemulsion method to three kinds of QDs with different structure: CdSe core and 2 nm CdS shell (CdSe/CdS-thin); CdSe core and 6 nm CdS shell (CdSe/CdS-thick); and CdS core, CdSe intermediate shell and 5 nm CdS outer shell (CdS/CdSe/CdS-SQW). Silica encapsulation inevitably results in lower photoluminescence quantum yield (PL QY) than pristine QDs due to formation of surface defects. However, the retaining ratio of pristine QY is different in the three silica coated samples; for example, CdSe/CdS-thin/SiO<SUB>2</SUB> shows the lowest retaining ratio (36%) while the retaining ratio of pristine PL QY in CdSe/CdS-thick/SiO<SUB>2</SUB> and SQW/SiO<SUB>2</SUB> is over 80% and SQW/SiO<SUB>2</SUB> shows the highest resulting PL QY. Thick outermost CdS shell isolates the excitons from the defects at surface, making PL QY relatively insensitive to silica encapsulation. The bright SiO<SUB>2</SUB>-coated SQW sample shows robustness against harsh conditions, such as acid etching and thermal annealing. The high luminescence and long-term stability highlights the potential of using the SQW/SiO<SUB>2</SUB> nanoparticles in bio-labeling or display applications.</P>
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Effect of Action Observational Training on Gait in People with Stroke
Lee, JongSu,Kim, YoungMi,Lee, DongKyu 대한물리치료학회 2020 대한물리치료학회지 Vol.32 No.1
Purpose: This study examined the effects of action observational training to improve the gait function for patients with stroke. Methods: The participants were divided into two groups: right hemiplegia group (n=12) and left hemiplegia group (n=12). All groups received conventional therapy for five sessions for 30 minutes, each for three weeks. Left and right hemiplegia group practiced additional action observational training for five sessions for 20 minutes each for three weeks. They participated in three weeks of action observational training coupled with immediate physical practice (intervention), followed by a final assessment. The duration of each action observation video sequence was 10 minutes, followed immediately by practice of the observed motor skill (10 minutes). The gait velocity, cadence, swing time, step length, and BOS (base of support) were examined using the GAITRite system. Results: The results of this study showed significant improvement in the gait function. The outcomes of the gait abilities from gait velocity, cadence, swing time, step length of the affected side, and BOS (base of support) were improved significantly in the right hemiplegia group (p<0.05). In the left hemiplegia group, there was no significant improvement in the gait velocity, cadence, and BOS except for the swing time and step length of the affected side. The left and right group comparisons between the groups were not significant (p<0.05). Conclusion: Action observation training improves the gait function. These results suggest that action observational training is feasible and suitable for stroke patients.
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Dongkyu Lee,Youngeun Kim,Oh Hyeong Kwon,Won Ho Park,Donghwan Cho 한국탄소학회 2021 Carbon Letters Vol.31 No.3
The effect of multi-walled carbon nanotubes (MWCNT) coating in the presence of polyethyleneimine (PEI) of different molecular weights (MW) on the interfacial shear strength (IFSS) of carbon fiber/acrylonitrile–butadiene–styrene (ABS) and carbon fiber/epoxy composites was investigated. The IFSS between the carbon fiber and the polymer was evaluated by means of single fiber microbonding test. The results indicated that uses of the carbon fibers uncoated and coated with pristine, low MW PEI-treated, and high MW PEI-treated MWCNT significantly influenced the IFSS of both thermoplastic and thermosetting carbon fiber composites as well as the carbon fiber surface topography. The incorporation of low MW (about 1300) PEI into the carboxylated MWCNT was more effective not only to uniformly coat the carbon fiber with the MWCNT but also to improve the interfacial bonding strength between the carbon fiber and the polymer than that of high MW (about 25,000) PEI. In addition, carbon fiber/epoxy composite exhibited the IFSS much higher than carbon fiber/ABS composite due to the chemical interactions between the epoxy resin and amine groups existing in the PEI-treated MWCNT.
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Dongkyu Lee,Kwanghyun Kim,Youngrong Lee,Kyungwon Oh,정선재 대한예방의학회 2022 예방의학회지 Vol.55 No.6
Objectives: Thiamine is thought to modify sleeping patterns, while alcohol use diminishes internal thiamine levels. We investigated the association between thiamine intake and sleep duration and explored possible heterogeneity in the effect according to alcohol use. Methods: In total, 15 384 participants aged 19-64 were obtained from the Korea National Health and Nutrition Examination Survey 2012-2016. Nutrient intake, including thiamine, was measured using a food frequency questionnaire. Sleep duration was measured by a self-reported questionnaire. The highest thiamine intake quartile was set as the reference group. Participants were divided into 3 groups, with 7-8 hours of daily sleep as a reference group and those who slept more or less than that as “oversleeping” and “insufficient sleeping,” respectively. Multivariate logistic regression was used, adjusting for socioeconomic, medical, and nutritional factors. Additionally, participants were stratified according to high-risk alcohol use defined by the World Health Organization standards on alcohol use. Results: Low thiamine intake was associated with oversleeping (Q3: odds ratio [OR], 1.06; 95% confidence interval [CI], 0.86 to 1.32; Q2: OR, 1.24; 95% CI, 0.99 to 1.55; Q1: OR, 1.49; 95% CI, 1.16 to 1.91) and showed a significant trend for higher ORs at lower intake levels (p-trend<0.001). The effect was stronger in the high-risk alcohol use group (Q1: OR, 1.78; 95% CI, 1.28 to 2.49). Conclusions: Low thiamine intake was associated with oversleeping, and alcohol use intensified that association. These results were found in a context where overt clinical symptoms due to thiamine deficiency are considered rare. More awareness of the potential relationship of thiamine intake with oversleeping and its related risks should be considered.
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